heal.abstract |
We have computed multiphoton ionization rates for He irradiated by a dichromatic ac field consisting of the fundamental wavelength λ = 248 nm and its second-, third-, and fourth-higher harmonics. The intensities are in the range 1.0 × 1012 - 3.5 × 1014 W/cm2, with the intensity of the harmonics being 1-2 orders of magnitude smaller. The calculations incorporated systematically electronic structure and electron correlation effects in the discrete and in the continuous spectrum, for1S,1P,1D,1F,1G, and1H two-electron states of even and odd parity. They were done by implementing a time-independent, nonperturbative many-electron, many-photon theory which obtains cycle-averaged complex eigenvalues, whose real part gives the field-induced energy shift, Δ(ω1,F1;ω2,F2,φ2), and the imaginary part is the multiphoton ionization rate, Γ(ω1,F1;ω2,F2,φ2), where ω is the frequency, F is the field strength, and φ2 is the phase difference. Through analysis and computation we show that, provided the intensities are weak, the dependence of Γ(ω1,F1;ω2,F2,φ2) on φ2 is simple. Specifically, for odd higher harmonics, Γ varies linearly with cos(φ2) whilst for even higher harmonics it varies linearly with cos(2φ2). These relations may turn out to be applicable to other atomic systems as well, and to provide a definition of the weak-field regime in the dichromatic case. When the combination of (ω1,F1) and (ω2,F2) is such that higher powers of cos(φ2) and cos(2φ2) become important, these rules break down and we reach the strong-field regime. ©2000 The American Physical Society. |
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