heal.abstract |
We have computed multiphoton ionization rates for He irradiated by a dichromatic ac held consisting of the fundamental wavelength lambda = 248 nm and its second-, third-, and fourth-higher harmonics. The intensities are in the range 1.0 x 10(12)-3.5 x 10(14) W/cm(2), with the intensity of the harmonics being 1-2 orders of magnitude smaller. The calculations incorporated systematically electronic structure and electron correlation effects in the discrete and in the continuous spectrum, for S-1, P-1, D-1, F-1, (1)G, and H-1 two-electron states of even and odd parity. They were done by implementing a time-independent, nonperturbative many-electron, many-photon theory which obtains cycle-averaged complex eigenvalues, whose real part gives the field-induced energy shift, Delta (w(1).F-1;omega (2),F-2,phi (2)), and the imaginary part is the multiphoton ionization rate, Gamma(omega (1),F-1;omega (2),F-2,phi (2)), where omega is the frequency. F is the field strength, and phi (2) is the phase difference. Through analysis and computation we show that, provided the intensities are weak, the dependence of Gamma(omega (1),F-1;omega (2),F-2,phi (2)) on phi (2) is simple. Specifically, for odd higher harmonics, Gamma varies linearly with cos(phi (2)) whilst for even higher harmonics it varies linearly with cos(2 phi (2)). These relations may turn out to be applicable to other atomic systems as well, and to provide a definition of the weak-field regime in the dichromatic case. When the combination of (omega (1),F-1) and (omega (2),F-2) is such that higher powers of cos(omega (2)) and cos(2 omega (2)) become important, these rules break down and we reach the strong-field regime. |
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